In the simple keyword search box, you can put such words after S: in order to specify the SUBJECT field.
ex.: "labor history" and S:sources
In the advanced keyword search, you can put your search term(s) in the top box, and in the second box, put the word(s) you're using to locate primary sources in the next box, and change the drop-down menu to Subject:
Keywords that will help you find primary sources:
Depending on the period being studied, it can also be helpful to limit your search by publication date.
More keywords identifying primary sources in Library of Congress Subject Headings